What about Clayface, Manbat, Bane, Hugo Strange, Ra's al Ghoul and many others while he was a meber in the Justice League
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Spiderman.
The original movies, and superhero movies in general, back then, were pretty lousy. They were basically campy to no end, because America as a general rule tend to view comics and cartoons as a primarily childish endeavor and thus all mainstream media tends to reflect this stereotype.
I really REALLY liked 'Batman: The Animated Series' in part due to my complain illustrated in the previous paragraph.
I don't remember much about Superman movies except that he flew 'backwards' and reversed time somehow, fought a hacker, and then fought Nuclear Man. Yes I only recall the sequels. No wonder I don't like Chris Reeves Superman.