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Mix is definitely the best for me, because I unlocked 60 Three Stars from the Monster Arena (I think you get them for capturing every monster on Gagazet, not sure though), and two of them gives you Sunburst/Supernova, which by the end of the game was the best overdrive for me (excluding aeon overdrives). I also liked Grand Summon, it really helps during tough bosses. Banishing Blade had awesome effects, although I could never get the button combo in time. Ronso Rages are cool too.
Blitz Ace, Mega Flare, and Oblivion.
Blitz Ace and Banishing Blade
oooOh I also like Rikku's mixing.
I think I liked Blitz Ace the best because Auron, Lulu, Wakka, Rikku, Yuna, or Kimahri can pass him the blitzball, depending on who you talk to first (or the most) or who you heal the most with Tidus. That was awesome.
I kinda liked Seymour's overdrive. It's a pain in the neck to wait for his Overdrive to fill but I had to see it once.
Oblivion was amazing.
I like Blitz Ice too.
I wasn't really impressed by anybody's overdrives... I guess I liked all of Auron's though.
I had only 2 of aurons overdrive
Oblivition, Fury. May be I'll like the nova too...