I don't watch a whole lot of anime but there's a handful that I really really like.

Noein
Dragon Ball-Z-GT
Escaflowne
Full Metal Alchemist
Cowboy Bebop
Neon Genesis Evangelion
Akira
anything from Hayao Miyazaki

FF Unlimited was okay. Didn't really like the switching back and forth of the animation styles, and if that wasn't what it was then my eyes are smurfed up.