Health Ledger is so far and above everyone else, that the real battle is for second best performance. For me, those contestants are:
RDJ as Iron Man
Jackie Earl Haley as Rorschach
Hugo Weaving as V
Possibly some others I'm forgetting. And even though it was a less serious role, I have to give credit for J.K. Simmons as J. Jonah Jameson (the best part of the original Spider-Man trilogy).
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