I could see a Marvel Cinematic Universe type thing going with FF6 since everyone in it has a unique power and backstory you could create an individual origin story for half the characters character (maybe joint movies for Edgar/Sabin, Strago/Relm/Shadow, Terra/Celes) and tie it all up with a Returners movie. for the World of Balance, and a stage 2 movie series for the World of Ruin.
If it had to be a whole FF condensed into one 2 - 3.5 hour movie then maybe FF13 since that seems to have the most simplistic, easily condensed story. If it was directed with the finesse of Mad Max 4 and had well choreographed well shot mind blowing action with subtle character development throughout it could be great.
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