Compete Series/Movie/OAV Set:
DNA<sup>2</sup>
Love Hina
Love Hina Again
Ah! Megami-sama/Oh! My Goddess OAV
Ah! Megami-sama/Oh! My Goddess Movie
Neon Genesis Evangelion
Neon Genesis Evangelion: Death and Rebirth
The End of Evangelion
Saishuuheiki Kanojo/She, The Ultimate Weapon
Angelic Layer
Boogiepop Phantom
Kare Kano/His and Her Circumstances
Serial Experiments Lain
Yokohama Kaidashi Kikou/Quiet Country Cafe OAV
First Kiss Story OAV
Furi Kuri
Onegai Teacher
Onegai Twins
Ranma 1/2: An Akane to Remember OAV
Record of Lodoss War
If I See You in My Dreams OAV
sCRYed
Welcome to Pia Carrot 2 Dx
Pia Carrot the Movie
Porco-Rosso
Sister Princess RePure
Star Ocean Ex
Neko no Ongaeshi/The Cat Returns
Flame of Recca
Chobits
Boys Be
Me Neighbor Totoro
Haibane Renmei
Hellsing
Azumanga Daioh
Read or Die OAV
3x3 Eyes

Incomplete:
Gunslinger Girls
Sailormoon (I have most)
Knights of Ramune
Sakura Diaries
Tenchi Universe
Dirty Pair

I want but am too lazy to get:
I Me My! Strawberry Eggs
Hand Maid May
Excel Saga
Final Fantasy Unlimited
Ayashi no Ceres
D.N.Angel
Fruit Basket
Noir
.hack//SIGN
Hana Yori Dango (+movie)

I also have 15GB of manga and about 30 graphic novels 'cause manga is hot.