(Legal) DVDs:
Cowboy Bebop (1-26)
Cowboy Bebop, the movie.
Records of Lodoss Wars (haven't watched that in a while, now that I think about it).
Serial Experiments Lain (4 DVDs)
Kiki's delivery service.
Spirited Away
Mononoke Hime
Laputa, the castle in the sky.
The kingdom of Cats (can't remember what the exact English title is).
Les triplettes de Belleville.
Ghost in the Shell
GitS: Innocence.
Ghost in the Shell: SAC (DVDs 1-5, about to get #6)
Kenshin OAV1 (will be getting the second OAV when it's out later this month)
Kenshin TV (DVDs 1-3, I ought to get the others someday)
Gunnm
Blood: the last vampire
Akira
Animatrix
Iria (3 DVDs)
D.N.A˛ (DVDs 1 & 2)

Legal VHS:
Magic Knight Rayearth Season 1
Parts of MK Rayearth Season 2
Lodoss War TV

On the comp/Burned on CDs/DVDs:
Trigun
Ah! My goddess OAV1
Ah! My Goddess ep 1-12
Naruto ep 1-146
Naruto the movie #1
Elfen Lied ep 1-3
.hack//SIGN
Ragnarök Online (I think I burned them, no clue where the CDs/DVD are now).
Escaflowne, the movie.
Saint Seyia Hades - Special
Saint Seyia Hades OVA 1-13
Saint Seyia - Stairway to heaven.
Tenju Tenge 1-24 & OVA1
Blame! Log 1-5 + Extra Log
FLCL
Noir